- Open Access
Thermalization of strongly interacting bosons after spontaneous emissions in optical lattices
© Schachenmayer et al.; licensee Springer on behalf of EPJ 2014
- Received: 1 August 2014
- Accepted: 7 November 2014
- Published: 4 January 2015
We study the out-of-equilibrium dynamics of bosonic atoms in a 1D optical lattice, after the ground-state is excited by a single spontaneous emission event, i.e. after an absorption and re-emission of a lattice photon. This is an important fundamental source of decoherence for current experiments, and understanding the resulting dynamics and changes in the many-body state is important for controlling heating in quantum simulators. Previously it was found that in the superfluid regime, simple observables relax to values that can be described by a thermal distribution on experimental time-scales, and that this breaks down for strong interactions (in the Mott insulator regime). Here we expand on this result, investigating the relaxation of the momentum distribution as a function of time, and discussing the relationship to eigenstate thermalization. For the strongly interacting limit, we provide an analytical analysis for the behavior of the system, based on an effective low-energy Hamiltonian in which the dynamics can be understood based on correlated doublon-holon pairs.
- optical lattices
- spontaneous emissions
- Bose-Hubbard model
An important fundamental question in many-body quantum mechanics is to what extent and under which conditions an isolated system perturbed away from equilibrium will undergo thermalization, in the sense that at long times the system will reach a steady state where simple observables equal the values for a thermal distribution [1–5]. Recently it has been possible to observe integrable dynamics for strongly interacting cold gases confined to move in one dimension , and thus reach regimes where systems either do not thermalize in this standard sense  or otherwise undergo generalized thermalization [8, 9].
These fundamental questions also have an important impact on the application of cold atoms as quantum simulators [10, 11]. Development in experiments with these systems has reached a stage where it is possible to tailor interesting many-body Hamiltonians, and study the many-body physics of corresponding ground states. However, some of the most interesting physical regimes require the realization of states with small energy gaps, requiring exceptionally low temperatures and entropies, which provide a key challenge for current experiments . This has been particularly true in attempts to observe quantum magnetism in optical lattices within strongly interacting regimes , where U is the on-site interaction energy, and indicates the tunneling amplitude for particles moving between neighboring sites. There, magnetic order in multi-species mixtures is driven by terms of the order of , which is typically small for current experiments [12–19].
In this context, it is very important to understand and control the many-body effects of competing heating processes in experiments. Previously, it has often been assumed that all of the energy added to the system will be thermalized, causing an effective increase in temperature. However, in regimes in which the system does not thermalize excitations entirely (or for some types of excitations, at all), the behavior is more complex. A simple example where excitations cannot thermalize on typical experimental timescales is given by spontaneous emission events (incoherent light scattering). In such processes, the main contribution to the increase in the average energy of the system as a function of time comes from atoms being excited to higher Bloch bands of an optical lattice [20–23]. Because the bandgap is usually much larger than the typical energy scales U and J of dynamics in the lowest band, it is not possible for the system to thermalize most of the energy added to the system as a function of time.
At the same time, understanding this process is made more complex by the fact that processes exciting particles to higher Bloch bands are rare compared with processes leaving particles in the lowest band in typical experiments [20, 21]. As a result, the dynamics can actually be dominated by heating in the lowest band of the lattice, the basic effects of which have been studied in several recent articles for bosons [20, 21, 24–28] and for fermions [29–31]. It is then natural to ask, in particular, whether the system can thermalize after spontaneous emission events that leave atoms in the lowest band.
In this article, we study the interplay between spontaneous emissions and thermalization in detail, asking under what conditions key simple quantities such as the quasimomentum distribution and the kinetic energy relax to values given by a thermal distribution. In each case, we ask this question in a practical context by fixing a thermal distribution such that we take a canonical ensemble with the temperature T chosen so that the expectation value of the energy in the thermal distribution matches the expectation value of the energy after a spontaneous emission event. In the case of strong interactions, we might expect that the system reaches integrable limits where the system does not thermalize. On the other hand, one might also expect that as in general, the Bose-Hubbard Hamiltonian is non-integrable, that outside the special cases of strong interactions ( ) and non-interacting systems ( ), thermalization would essentially always occur.
Instead, we find that this generalization is not universally applicable. It is important to note that spontaneous emissions correspond to local quenches for the many-body state, leading to population of low-lying excited states. As we showed previously , after a spontaneous emission, depending on the parameter regime and the corresponding different characteristics of the low-energy spectrum: either (i) the system relaxes over short times to thermal values of the quasimomentum distribution and kinetic energy, or (ii) on short timescales, the system relaxes to states that are clearly non-thermal, even if all atoms remain in the lowest Bloch band. The latter regime was found to occur if the interactions are strong enough so that the ground-state of the system corresponds to a Mott insulator state. Below we elaborate on these results especially for the quasimomentum distribution, and discuss their interpretation in terms of eigenstate thermalization.
In the limit where the system is close to an ideal Mott-insulator (a product state with a fixed number of particles per cite) and in the case of unit filing, one can describe the dynamics of the system in an effective model, where one restricts the local Hilbert space to having a maximum of two particles per site. The low-lying excitations can then be described as correlated pairs of holes (“holons”) and doubly occupied sites (“doublons”) [26, 32]. Here we use this approximation to show that no thermalization is present for spontaneous emission in this limit. We compare our result to exact numerical calculations either using exact diagonalization in small systems, or by making use of t-DMRG techniques [33–36].
This article is organized as follows. We begin by introducing spontaneous emissions and thermalization in these systems in Section 2. Then, in Section 3 we review the explanation of the basic behavior we find in terms of the eigenstate thermalization. In Section 4 we discuss how the behavior can be understood in the strongly interacting limit, making predictions that could be observed for the propagation of excitations when the system does not thermalize in that limit. In Section 5 we then provide a summary and outlook.
Spontaneous emissions are a fundamental source of heating in optical dipole potentials [22, 23], and one of the key contributing heating sources in current experiments with cold atoms in optical lattices [20, 21]. As shown in Ref. , a multi-band many-body master equation can be derived to describe this process in the case of far detuned lattice light. An adiabatic elimination of the electronic excited states leads to an equation for atoms in their electronic ground states. Taking this, and assuming the typical experimental case in which the lattice spacing a is comparable to the wavelength of scattered photons, , the dynamics of the many-body density operator ρ follows a master equation of the form ( ), . Here is a multi-band Bose-Hubbard Hamiltonian and includes dissipative Lindblad terms with on-site jump operators . Here, is the bosonic annihilation operator at site i, for a particle in band m.
In the following we will focus on a system with M sites and particles, so that the filling is . In this case the system undergoes a ground-state quantum phase transition between a superfluid (SF) and a Mott insulating (MI) state at the critical value, which was estimated to be [37, 38]. The underlying physics of the lattice-photon scattering process can be summarized as the environment obtaining information about the position of an atom. Thereby the atoms are localized on the length-scale of a single lattice-site size.
Here, we demonstrate a specific example of this in Figures 1(e),(f). There we show relaxation of a high-q component of the quasimomentum distribution, , in a system with lattice sites. We can clearly see that after a short period of time, this component relaxes to its value in a corresponding thermal distribution provided that we initially start in a superfluid state with . In the MI limit, we see that the behavior is similar, in so far as there is a rapid relaxation of this value of quasimomentum on short times. However, this leads to a value that is markedly different to the corresponding thermal value. It is naturally possible that in this regime, there are processes on very long timescales that will eventually lead to thermalization of this quantity. But it is clear that on the MI side of the phase transition, the system exhibits a qualitatively different behavior in terms of how close it is to thermal distributions on the scale of a few tunnelling times. This will significantly impact the ability of the system to thermalize energy added by heating on the timescales of the heating process itself.
We note that the relaxation of the quasimomentum distribution could be directly observed (and compared to a thermal distribution) in a realistic experiment. Here one could use a near-resonant laser beam that is switched on for a particular time and provides the necessary heating through spontaneous emissions. In contrast to our calculations such an experiment would not be limited to relatively low heating rates, i.e. a small number of single spontaneous emissions. Thus, the discrepancies in the tails of the quasimomentum distribution from thermal values can be significantly larger than for the single spontaneous emission event considered in Figures 1(e),(f).
where denotes the ground-state of the system, and then take a stochastic average over the sites l, which is weighted proportional to the square of the density on site l, . The mechanism of this thermalization of closed quantum systems can be explained via eigenstate thermalizaton, a mechanism which we will review in the next section.
Thus, the value of the steady state expectation (if such a steady state is developed) only depends on two variables: (i) The expansion coefficients of the initial state, , and (ii) the expectation values of the energy-eigenstates with the particular observable, . The eigenstate thermalization hypothesis states, that if the eigenenergy expectation values of an observable vary smoothly in the energy window defined by the (and the off-diagonal , are small), the system relaxes into a state for which the observable can be described with a micro-canonical ensemble [1, 2].
In addition we plot a direct comparison of the two expectation values in Figure 2(d). We can calculate the expectation value on the one hand from the diagonal ensemble and on the other hand from a canonical ensemble with the same mean-energy. As initial state we choose the state after a single spontaneous emission on site . Although finite size effects play an important role in this small system, it is already obvious that a discrepancy between the two ensembles arises when entering the MI regime. As was found by t-DMRG calculations in , this also holds for larger systems. In the next section we will calculate the low-lying energy eigenstates exactly analytically in the limit of large interactions in the thermodynamic limit.
In this section we will discuss how we can understand the dynamics analytically for the case of strong interactions. In the extreme case of infinite U, at unit filling the particles will be in an idealized Mott insulator state, i.e., . This state is an eigenstate of the jump operator with eigenvalue one, so that light scattering leaving particles in the lowest band does not change the state or introduce any extra energy to the system. Naturally this is a trivial limit that is typically not reached in experiments, and we go beyond this below by considering situations where the amplitude for particles to be found on neighbouring sites is non-zero in the initial state, and light scattering can lead to the formation of pairs consisting of a doubly occupied site and a hole (unoccupied site).
4.1 Hard-core bosons
and the ground-state takes the product form (where denotes the state of a particle at site i). The jump-operators - as is true for all site-local operators - are unaffected by the Jordan-Wigner transformation and so in this transformed notation, .
If the system has fewer particles than lattice sites, spontaneous emissions will give rise to heating in the lowest band, as the states are not eigenstates of , which does not commute with the Hamiltonian. Simple results in this case are discussed in Ref. . However, in the special case of unit filling, which we would like to treat here, the only state described by this simple HCB form is again the trivial state with a single particle on each site, which is an eigenstate of all operators and . It is then clear that we need to go beyond this treatment in order to understand heating in a Mott Insulator state with finite U.
4.2 Doublon/holon calculation
4.3 Spontaneous emission in the doublon/holon picture
4.4 Behaviour of the kinetic energy and similar variables
where . Thus, we conclude that after a single spontaneous emission, observables of the form (24) can immediately be described by the diagonal ensemble, i.e. the effective density matrix for those observables takes a diagonal form in the basis low-lying energy states.
We compare this analytical result to our time-dependent t-DMRG calculations This is in excellent agreement with our numerical results even for relatively small as shown in Figure 4(b).
4.5 Eigenstate expectation values
In summary, we have investigated the non-equilibrium dynamics of bosons in an optical lattice in the presence of spontaneous emission events. We show clearly parameter regimes in which the system relaxes to thermal distributions for simple quanitites (especially the quasimomentum distribution), and others where it relaxes on short timescales to non-thermal values. We can understand this behavior by applying eigenstate thermalization considerations to small systems for which we can perform exact diagonalization calculations. We also show that we can understand the dynamics in the strongly interacting limit well in terms of propagating doublon-hole pairs, which are analytically tractable.
All of these results are expected to be directly observable in ongoing experiments. In addition to the possibility to measure quasimomentum distributions, the propagation of doublon-holon pairs as investigated here is a key signature for the effects of spontaneous emissions that could be measured in quantum gas microscope experiments with single-site resolution in ways that were previously implemented for quenches within the MI regime . Measurements of this type could be used as a diagnostic tool for heating of many-body states in optical lattices, which could in turn be used to improve the robustness of quantum simulators. In the future, these studies can be continued towards thermalization for fermions in optical lattices undergoing spontaneous emissions [29–31], and the incorporation of partial thermalization from excitations to higher Bloch bands.
We would like to thank I. Bloch, W. Ketterle, S. Langer, H. Pichler, U. Schneider, and P. Zoller for discussions. This work was supported in part by AFOSR grant FA9550-13-1-0093, by a grant from the US Army Research Office with funding from the DARPA OLE program, and by the Aspen Center for Physics support under NSF grant 1066293. JS was financially supported by NSF grants JILA-NSF-PFC-1125844 and NSF-PIF- 1211914. MT was supported by ERC Advanced Grant SIMCOFE and by the Swiss National Science Foundation through the National Competence Center in Research QSIT. Computational resources were provided by the Center for Simulation and Modeling at the University of Pittsburgh.
- Deutsch JM: Phys. Rev. A. 1991,43(4):2046. 10.1103/PhysRevA.43.2046View ArticleADSMathSciNetGoogle Scholar
- Srednicki M: Phys. Rev. E. 1994, 50:888.View ArticleADSGoogle Scholar
- Rigol M, Dunjko V, Olshanii M: Nature. 2008,452(7189):854. 10.1038/nature06838View ArticleADSGoogle Scholar
- Cazalilla MA, Citro R, Giamarchi T, Orignac E, Rigol M: Rev. Mod. Phys.. 2011, 83:1405. 10.1103/RevModPhys.83.1405View ArticleADSGoogle Scholar
- Rigol M, Srednicki M: Phys. Rev. Lett.. 2012., 108: Article ID 110601Google Scholar
- Kinoshita T, Wenger T, Weiss DS: Nature. 2006,440(7086):900. 10.1038/nature04693View ArticleADSGoogle Scholar
- Rigol M: Phys. Rev. Lett.. 2009., 103: Article ID 100403Google Scholar
- Cassidy AC, Clark CW, Rigol M: Phys. Rev. Lett.. 2011., 106: Article ID 140405Google Scholar
- Rigol M, Fitzpatrick M: Phys. Rev. A. 2011., 84: Article ID 033640Google Scholar
- Bloch I, Dalibard J, Nascimbene S: Nat. Phys.. 2012,8(4):267. 10.1038/nphys2259View ArticleGoogle Scholar
- Cirac JI, Zoller P: Nat. Phys.. 2012,8(4):264. 10.1038/nphys2275View ArticleGoogle Scholar
- McKay DC, DeMarco B: Rep. Prog. Phys.. 2011.,74(5): Article ID 054401Google Scholar
- Jördens R, Tarruell L, Greif D, Uehlinger T, Strohmaier N, Moritz H, Esslinger T, De Leo L, Kollath C, Georges A, Scarola V, Pollet L, Burovski E, Kozik E, Troyer M: Phys. Rev. Lett.. 2010.,104(18): Article ID 180401Google Scholar
- Hofstetter W, Cirac JI, Zoller P, Demler E, Lukin MD: Phys. Rev. Lett.. 2002.,89(22): Article ID 220407Google Scholar
- Mathy CJM, Huse DA, Hulet RG: Phys. Rev. A. 2012., 86: Article ID 023606Google Scholar
- Jördens R, Strohmaier N, Günter K, Moritz H, Esslinger T: Nature (London). 2008,455(7210):204. 10.1038/nature07244View ArticleADSGoogle Scholar
- Paiva T, Scalettar R, Randeria M, Trivedi N: Phys. Rev. Lett.. 2010., 104: Article ID 066406Google Scholar
- De Leo L, Bernier JS, Kollath C, Georges A, Scarola VW: Phys. Rev. A. 2011., 83: Article ID 023606Google Scholar
- Fuchs S, Gull E, Pollet L, Burovski E, Kozik E, Pruschke T, Troyer M: Phys. Rev. Lett.. 2011., 106: Article ID 030401Google Scholar
- Gerbier F, Castin Y: Phys. Rev. A. 2010., 82: Article ID 013615Google Scholar
- Pichler H, Daley AJ, Zoller P: Phys. Rev. A. 2010.,82(6): Article ID 063605Google Scholar
- Gordon JP, Ashkin A: Phys. Rev. A. 1980, 21:1606. 10.1103/PhysRevA.21.1606View ArticleADSGoogle Scholar
- Dalibard J, Cohen-Tannoudji C: J. Phys. B, At. Mol. Opt. Phys.. 1985,18(8):1661. 10.1088/0022-3700/18/8/019View ArticleADSMathSciNetGoogle Scholar
- Schachenmayer J, Pollet L, Troyer M, Daley AJ: Phys. Rev. A. 2014.,89(1): Article ID 011601Google Scholar
- Poletti D, Bernier JS, Georges A, Kollath C: Phys. Rev. Lett.. 2012., 109: Article ID 045302Google Scholar
- Barmettler P, Poletti D, Cheneau M, Kollath C: Phys. Rev. A. 2012.,85(5): Article ID 053625Google Scholar
- Poletti D, Barmettler P, Georges A, Kollath C: Phys. Rev. Lett.. 2013., 111: Article ID 195301Google Scholar
- arXiv: 1405.5404
- Bernier JS, Barmettler P, Poletti D, Kollath C: Phys. Rev. A. 2013., 87: Article ID 063608Google Scholar
- Sarkar S, Langer S, Schachenmayer J, Daley AJ: Phys. Rev. A. 2014.,90(2): Article ID 023618Google Scholar
- arXiv: 1407.1098
- Cheneau M, Barmettler P, Poletti D, Endres M, Schauß P, Fukuhara T, Gross C, Bloch I, Kollath C, Kuhr S: Nature. 2012,481(7382):484. 10.1038/nature10748View ArticleADSGoogle Scholar
- Vidal G: Phys. Rev. Lett.. 2004.,93(4): Article ID 040502Google Scholar
- Daley AJ, Kollath C, Schollwöck U, Vidal G: J. Stat. Mech. Theory Exp.. 2004., 2004: Article ID P04005Google Scholar
- White SR, Feiguin AE: Phys. Rev. Lett.. 2004.,93(7): Article ID 076401Google Scholar
- Verstraete F, Murg V, Cirac JI: Adv. Phys.. 2008, 57:143. 10.1080/14789940801912366View ArticleADSGoogle Scholar
- Schönmeier-Kromer J, Pollet L: Phys. Rev. A. 2014., 89: Article ID 023605Google Scholar
- Kühner TD, White SR, Monien H: Phys. Rev. B. 2000., 61: Article ID 12474Google Scholar
- Daley AJ: Adv. Phys.. 2014,63(2):77. 10.1080/00018732.2014.933502View ArticleADSGoogle Scholar
- Mølmer K, Castin Y, Dalibard J: J. Opt. Soc. Am. B. 1993,10(3):524. 10.1364/JOSAB.10.000524View ArticleADSGoogle Scholar
- Gardiner CW, Zoller P: Quantum Noise. Springer, Berlin; 2005.Google Scholar
- Carmichael HJ: An Open Systems Approach to Quantum Optics. Springer, Berlin; 1993.MATHGoogle Scholar
- Linden N, Popescu S, Short AJ, Winter A: Phys. Rev. E. 2009.,79(6): Article ID 061103Google Scholar
- Rigol M, Muramatsu A: Phys. Rev. A. 2004.,70(3): Article ID 031603Google Scholar
- Jordan P, Wigner E: Z. Phys.. 1928, 47:631. 10.1007/BF01331938View ArticleADSMATHGoogle Scholar
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